2024
|
18. | Dandan Hui; Husain Alqattan; Mohamed Sennary; Nikolay V Golubev; Mohammed Th Hassan: Attosecond electron microscopy and diffraction. In: Science Advances, vol. 10, no. 34, pp. eadp5805, 2024. @article{pmid39167650,
title = {Attosecond electron microscopy and diffraction},
author = {Dandan Hui and Husain Alqattan and Mohamed Sennary and Nikolay V Golubev and Mohammed Th Hassan},
doi = {10.1126/sciadv.adp5805},
year = {2024},
date = {2024-08-01},
urldate = {2024-08-01},
journal = {Science Advances},
volume = {10},
number = {34},
pages = {eadp5805},
abstract = {Advances in attosecond spectroscopy have enabled tracing and controlling the electron motion dynamics in matter, although they have yielded insufficient information about the electron dynamic in the space domain. Hence, ultrafast electron and x-ray imaging tools have been developed to image the ultrafast dynamics of matter in real time and space. The cutting-edge temporal resolution of these imaging tools is on the order of a few tens to a hundred femtoseconds, limiting imaging to the atomic dynamics and leaving electron motion imaging out of reach. Here, we obtained the attosecond temporal resolution in the transmission electron microscope, which we coined "attomicroscopy." We demonstrated this resolution by the attosecond diffraction measurements of the field-driven electron dynamics in graphene. This attosecond imaging tool would provide more insights into electron motion and directly connect it to the structural dynamics of matter in real-time and space domains, opening the door for long-anticipated real-life attosecond science applications in quantum physics, chemistry, and biology.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Advances in attosecond spectroscopy have enabled tracing and controlling the electron motion dynamics in matter, although they have yielded insufficient information about the electron dynamic in the space domain. Hence, ultrafast electron and x-ray imaging tools have been developed to image the ultrafast dynamics of matter in real time and space. The cutting-edge temporal resolution of these imaging tools is on the order of a few tens to a hundred femtoseconds, limiting imaging to the atomic dynamics and leaving electron motion imaging out of reach. Here, we obtained the attosecond temporal resolution in the transmission electron microscope, which we coined "attomicroscopy." We demonstrated this resolution by the attosecond diffraction measurements of the field-driven electron dynamics in graphene. This attosecond imaging tool would provide more insights into electron motion and directly connect it to the structural dynamics of matter in real-time and space domains, opening the door for long-anticipated real-life attosecond science applications in quantum physics, chemistry, and biology. |
2023
|
17. | Alan Scheidegger; Nikolay V. Golubev; Jiří Vaníček: How to Find Molecules with Long-lasting Charge Migration?. In: CHIMIA, vol. 77, no. 4, pp. 201, 2023. @article{ScheideggerChimia,
title = {How to Find Molecules with Long-lasting Charge Migration?},
author = {Alan Scheidegger and Nikolay V. Golubev and Jiří Vaníček},
doi = {https://doi.org/10.2533/chimia.2023.201},
year = {2023},
date = {2023-04-26},
journal = {CHIMIA},
volume = {77},
number = {4},
pages = {201},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2022
|
16. | Danylo T. Matselyukh; Victor Despré; Nikolay V. Golubev; Alexander I. Kuleff; Hans Jakob Wörner: Decoherence and revival in attosecond charge migration driven by non-adiabatic dynamics. In: Nature Physics, 2022. @article{Matselyukh2022,
title = {Decoherence and revival in attosecond charge migration driven by non-adiabatic dynamics},
author = {Danylo T. Matselyukh and Victor Despré and Nikolay V. Golubev and Alexander I. Kuleff and Hans Jakob Wörner},
doi = {https://doi.org/10.1038/s41567-022-01690-0},
year = {2022},
date = {2022-08-04},
journal = {Nature Physics},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
15. | Nikolay Golubev; Jiří Vaníček: Efficient Semiclassical Evaluation of Electronic Coherences in Polyatomic Molecules. In: Chimia, vol. 76, no. 6, pp. 575, 2022. @article{Golubev_review2022,
title = {Efficient Semiclassical Evaluation of Electronic Coherences in Polyatomic Molecules},
author = {Nikolay Golubev and Jiří Vaníček},
doi = {10.2533/chimia.2022.575},
year = {2022},
date = {2022-06-29},
journal = {Chimia},
volume = {76},
number = {6},
pages = {575},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
14. | Alan Scheidegger; Jiří Vaníček; Nikolay V. Golubev: Search for long-lasting electronic coherence using on-the-fly ab initio semiclassical dynamics. In: The Journal of Chemical Physics, vol. 156, no. 3, pp. 034104, 2022. @article{Scheidegger2022,
title = {Search for long-lasting electronic coherence using on-the-fly ab initio semiclassical dynamics},
author = {Alan Scheidegger and Jiří Vaníček and Nikolay V. Golubev},
doi = {https://doi.org/10.1063/5.0076609},
year = {2022},
date = {2022-01-18},
journal = {The Journal of Chemical Physics},
volume = {156},
number = {3},
pages = {034104},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2021
|
13. | Nikolay V. Golubev; Jiří Vaníček; Alexander I. Kuleff: Core-Valence Attosecond Transient Absorption Spectroscopy of Polyatomic Molecules. In: Phys. Rev. Lett., vol. 127, pp. 123001, 2021. @article{Golubev2021,
title = {Core-Valence Attosecond Transient Absorption Spectroscopy of Polyatomic Molecules},
author = {Nikolay V. Golubev and Jiří Vaníček and Alexander I. Kuleff},
doi = {10.1103/PhysRevLett.127.123001},
year = {2021},
date = {2021-09-16},
journal = {Phys. Rev. Lett.},
volume = {127},
pages = {123001},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2020
|
12. | Nikolay V. Golubev; Tomislav Begušić; Jiří Vaníček: On-the-Fly Ab Initio Semiclassical Evaluation of Electronic Coherences in Polyatomic Molecules Reveals a Simple Mechanism of Decoherence. In: Phys. Rev. Lett., vol. 125, pp. 083001, 2020. @article{Golubev2020,
title = {On-the-Fly Ab Initio Semiclassical Evaluation of Electronic Coherences in Polyatomic Molecules Reveals a Simple Mechanism of Decoherence},
author = {Nikolay V. Golubev and Tomislav Begušić and Jiří Vaníček},
doi = {10.1103/PhysRevLett.125.083001},
year = {2020},
date = {2020-08-17},
journal = {Phys. Rev. Lett.},
volume = {125},
pages = {083001},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2018
|
11. | Victor Despré; Nikolay V Golubev; Alexander I Kuleff: Charge Migration in Propiolic Acid: A Full Quantum Dynamical Study. In: Phys. Rev. Lett., vol. 121, pp. 203002, 2018. @article{PhysRevLett.121.203002,
title = {Charge Migration in Propiolic Acid: A Full Quantum Dynamical Study},
author = {Victor Despré and Nikolay V Golubev and Alexander I Kuleff},
doi = {10.1103/PhysRevLett.121.203002},
year = {2018},
date = {2018-11-01},
journal = {Phys. Rev. Lett.},
volume = {121},
pages = {203002},
publisher = {American Physical Society},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
10. | Y. Kumagai; H. Fukuzawa; K. Motomura; D. Iablonskyi; K. Nagaya; S. Wada; Y. Ito; T. Takanashi; Y. Sakakibara; D. You; T. Nishiyama; K. Asa; Y. Sato; T. Umemoto; K. Kariyazono; E. Kukk; K. Kooser; C. Nicolas; C. Miron; T. Asavei; L. Neagu; M. S. Schöffler; G. Kastirke; X. Liu; S. Owada; T. Katayama; T. Togashi; K. Tono; M. Yabashi; N. V. Golubev; K. Gokhberg; L. S. Cederbaum; A. I. Kuleff; K. Ueda: Following the Birth of a Nanoplasma Produced by an Ultrashort Hard-X-Ray Laser in Xenon Clusters. In: Phys. Rev. X, vol. 8, pp. 031034, 2018. @article{PhysRevX.8.031034,
title = {Following the Birth of a Nanoplasma Produced by an Ultrashort Hard-X-Ray Laser in Xenon Clusters},
author = {Y. Kumagai and H. Fukuzawa and K. Motomura and D. Iablonskyi and K. Nagaya and S. Wada and Y. Ito and T. Takanashi and Y. Sakakibara and D. You and T. Nishiyama and K. Asa and Y. Sato and T. Umemoto and K. Kariyazono and E. Kukk and K. Kooser and C. Nicolas and C. Miron and T. Asavei and L. Neagu and M. S. Schöffler and G. Kastirke and X. Liu and S. Owada and T. Katayama and T. Togashi and K. Tono and M. Yabashi and N. V. Golubev and K. Gokhberg and L. S. Cederbaum and A. I. Kuleff and K. Ueda},
doi = {10.1103/PhysRevX.8.031034},
year = {2018},
date = {2018-08-01},
journal = {Phys. Rev. X},
volume = {8},
pages = {031034},
publisher = {American Physical Society},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
9. | B. Schütte; C. Peltz; D. R. Austin; C. Strüber; P. Ye; A. Rouzée; M. J. J. Vrakking; N. Golubev; A. I. Kuleff; T. Fennel; J. P. Marangos: Low-Energy Electron Emission in the Strong-Field Ionization of Rare Gas Clusters. In: Phys. Rev. Lett., vol. 121, pp. 063202, 2018. @article{PhysRevLett.121.063202,
title = {Low-Energy Electron Emission in the Strong-Field Ionization of Rare Gas Clusters},
author = {B. Schütte and C. Peltz and D. R. Austin and C. Strüber and P. Ye and A. Rouzée and M. J. J. Vrakking and N. Golubev and A. I. Kuleff and T. Fennel and J. P. Marangos},
doi = {10.1103/PhysRevLett.121.063202},
year = {2018},
date = {2018-08-01},
journal = {Phys. Rev. Lett.},
volume = {121},
pages = {063202},
publisher = {American Physical Society},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2017
|
8. | Nikolay V Golubev; Victor Despré; Alexander I Kuleff: Quantum Control with Smoothly Varying Pulses: General Theory and Application to Charge Migration. In: Journal of Modern Optics, vol. 64, no. 10-11, pp. 1031–1041, 2017. @article{my_golubev2017qoc,
title = {Quantum Control with Smoothly Varying Pulses: General Theory and Application to Charge Migration},
author = {Nikolay V Golubev and Victor Despré and Alexander I Kuleff},
doi = {10.1080/09500340.2016.1275855},
year = {2017},
date = {2017-01-01},
urldate = {2017-10-23},
journal = {Journal of Modern Optics},
volume = {64},
number = {10-11},
pages = {1031--1041},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
7. | T. Takanashi; N. V. Golubev; C. Callegari; H. Fukuzawa; K. Motomura; D. Iablonskyi; Y. Kumagai; S. Mondal; T. Tachibana; K. Nagaya; T. Nishiyama; K. Matsunami; P. Johnsson; P. Piseri; G. Sansone; A. Dubrouil; M. Reduzzi; P. Carpeggiani; C. Vozzi; M. Devetta; M. Negro; D. Faccial`a; F. Calegari; A. Trabattoni; M. C. Castrovilli; Y. Ovcharenko; M. Mudrich; F. Stienkemeier; M. Coreno; M. Alagia; B. Schütte; N. Berrah; O. Plekan; P. Finetti; C. Spezzani; E. Ferrari; E. Allaria; G. Penco; C. Serpico; G. De Ninno; B. Diviacco; S. Di Mitri; L. Giannessi; G. Jabbari; K. C. Prince; L. S. Cederbaum; Ph. V. Demekhin; A. I. Kuleff; K. Ueda: Time-Resolved Measurement of Interatomic Coulombic Decay Induced by Two-Photon Double Excitation of Ne2. In: Phys. Rev. Lett., vol. 118, pp. 033202, 2017. @article{PhysRevLett.118.033202,
title = {Time-Resolved Measurement of Interatomic Coulombic Decay Induced by Two-Photon Double Excitation of Ne2},
author = {T. Takanashi and N. V. Golubev and C. Callegari and H. Fukuzawa and K. Motomura and D. Iablonskyi and Y. Kumagai and S. Mondal and T. Tachibana and K. Nagaya and T. Nishiyama and K. Matsunami and P. Johnsson and P. Piseri and G. Sansone and A. Dubrouil and M. Reduzzi and P. Carpeggiani and C. Vozzi and M. Devetta and M. Negro and D. Faccial`a and F. Calegari and A. Trabattoni and M. C. Castrovilli and Y. Ovcharenko and M. Mudrich and F. Stienkemeier and M. Coreno and M. Alagia and B. Schütte and N. Berrah and O. Plekan and P. Finetti and C. Spezzani and E. Ferrari and E. Allaria and G. Penco and C. Serpico and G. De Ninno and B. Diviacco and S. Di Mitri and L. Giannessi and G. Jabbari and K. C. Prince and L. S. Cederbaum and Ph. V. Demekhin and A. I. Kuleff and K. Ueda},
doi = {10.1103/PhysRevLett.118.033202},
year = {2017},
date = {2017-01-01},
journal = {Phys. Rev. Lett.},
volume = {118},
pages = {033202},
publisher = {American Physical Society},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
6. | M. C. E. Galbraith; S. Scheit; N. V. Golubev; G. Reitsma; N. Zhavoronkov; V. Despré; F. Lépine; A. I. Kuleff; M. J. J. Vrakking; O. Kornilov; H. Köppel; J. Mikosch: Few-femtosecond passage of conical intersections in the benzene cation. In: Nature Communications, vol. 8, no. 1, pp. 1018, 2017, ISSN: 2041-1723. @article{Galbraith2017,
title = {Few-femtosecond passage of conical intersections in the benzene cation},
author = {M. C. E. Galbraith and S. Scheit and N. V. Golubev and G. Reitsma and N. Zhavoronkov and V. Despré and F. Lépine and A. I. Kuleff and M. J. J. Vrakking and O. Kornilov and H. Köppel and J. Mikosch},
doi = {10.1038/s41467-017-01133-y},
issn = {2041-1723},
year = {2017},
date = {2017-01-01},
journal = {Nature Communications},
volume = {8},
number = {1},
pages = {1018},
abstract = {Observing the crucial first few femtoseconds of photochemical reactions requires tools typically not available in the femtochemistry toolkit. Such dynamics are now within reach with the instruments provided by attosecond science. Here, we apply experimental and theoretical methods to assess the ultrafast nonadiabatic vibronic processes in a prototypical complex system--the excited benzene cation. We use few-femtosecond duration extreme ultraviolet and visible/near-infrared laser pulses to prepare and probe excited cationic states and observe two relaxation timescales of 11 textpm 3 fs and 110 textpm 20 fs. These are interpreted in terms of population transfer via two sequential conical intersections. The experimental results are quantitatively compared with state-of-the-art multi-configuration time-dependent Hartree calculations showing convincing agreement in the timescales. By characterising one of the fastest internal conversion processes studied to date, we enter an extreme regime of ultrafast molecular dynamics, paving the way to tracking and controlling purely electronic dynamics in complex molecules.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
Observing the crucial first few femtoseconds of photochemical reactions requires tools typically not available in the femtochemistry toolkit. Such dynamics are now within reach with the instruments provided by attosecond science. Here, we apply experimental and theoretical methods to assess the ultrafast nonadiabatic vibronic processes in a prototypical complex system--the excited benzene cation. We use few-femtosecond duration extreme ultraviolet and visible/near-infrared laser pulses to prepare and probe excited cationic states and observe two relaxation timescales of 11 textpm 3 fs and 110 textpm 20 fs. These are interpreted in terms of population transfer via two sequential conical intersections. The experimental results are quantitatively compared with state-of-the-art multi-configuration time-dependent Hartree calculations showing convincing agreement in the timescales. By characterising one of the fastest internal conversion processes studied to date, we enter an extreme regime of ultrafast molecular dynamics, paving the way to tracking and controlling purely electronic dynamics in complex molecules. |
2016
|
5. | K Nagaya; D Iablonskyi; N V Golubev; K Matsunami; H Fukuzawa; K Motomura; T Nishiyama; T Sakai; T Tachibana; S Mondal; S Wada; K C Prince; C Callegari; C Miron; N Saito; M Yabashi; Ph. V Demekhin; L S Cederbaum; A I Kuleff; M Yao; K Ueda: Interatomic Coulombic decay cascades in multiply excited neon clusters. In: Nature Communications, vol. 7, pp. 13477, 2016. @article{Nagaya2016,
title = {Interatomic Coulombic decay cascades in multiply excited neon clusters},
author = {K Nagaya and D Iablonskyi and N V Golubev and K Matsunami and H Fukuzawa and K Motomura and T Nishiyama and T Sakai and T Tachibana and S Mondal and S Wada and K C Prince and C Callegari and C Miron and N Saito and M Yabashi and Ph. V Demekhin and L S Cederbaum and A I Kuleff and M Yao and K Ueda},
doi = {10.1038/ncomms13477},
year = {2016},
date = {2016-12-01},
journal = {Nature Communications},
volume = {7},
pages = {13477},
publisher = {Springer Nature},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2015
|
4. | Nikolay V Golubev; Alexander I Kuleff: Control of charge migration in molecules by ultrashort laser pulses. In: Phys. Rev. A, vol. 91, pp. 051401, 2015. @article{PhysRevA.91.051401,
title = {Control of charge migration in molecules by ultrashort laser pulses},
author = {Nikolay V Golubev and Alexander I Kuleff},
doi = {10.1103/PhysRevA.91.051401},
year = {2015},
date = {2015-05-01},
journal = {Phys. Rev. A},
volume = {91},
pages = {051401},
publisher = {American Physical Society},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2014
|
3. | Nikolay V Golubev; Alexander I Kuleff: Control of populations of two-level systems by a single resonant laser pulse. In: Phys. Rev. A, vol. 90, pp. 035401, 2014. @article{PhysRevA.90.035401,
title = {Control of populations of two-level systems by a single resonant laser pulse},
author = {Nikolay V Golubev and Alexander I Kuleff},
doi = {10.1103/PhysRevA.90.035401},
year = {2014},
date = {2014-09-01},
journal = {Phys. Rev. A},
volume = {90},
pages = {035401},
publisher = {American Physical Society},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2. | Éric Brémond; Nikolay Golubev; Stephan N Steinmann; Clémence Corminboeuf: How important is self-consistency for the dDsC density dependent dispersion correction?. In: The Journal of Chemical Physics, vol. 140, no. 18, pp. 18A516, 2014. @article{doi:10.1063/1.4867195,
title = {How important is self-consistency for the dDsC density dependent dispersion correction?},
author = {Éric Brémond and Nikolay Golubev and Stephan N Steinmann and Clémence Corminboeuf},
doi = {10.1063/1.4867195},
year = {2014},
date = {2014-01-01},
journal = {The Journal of Chemical Physics},
volume = {140},
number = {18},
pages = {18A516},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
2013
|
1. | Nikolay V Golubev; Dmitry S Bezrukov; Magnus Gustafsson; Gunnar Nyman; Sergey V Antipov: Formation of the SiP Radical through Radiative Association. In: The Journal of Physical Chemistry A, vol. 117, no. 34, pp. 8184-8188, 2013. @article{Golubev2013,
title = {Formation of the SiP Radical through Radiative Association},
author = {Nikolay V Golubev and Dmitry S Bezrukov and Magnus Gustafsson and Gunnar Nyman and Sergey V Antipov},
doi = {10.1021/jp403174u},
year = {2013},
date = {2013-01-01},
journal = {The Journal of Physical Chemistry A},
volume = {117},
number = {34},
pages = {8184-8188},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|